Structural instability at the In-terminated surface of the heavy-fermion superconductor CeIrIn5
Journal article, 2022

Driven by reconstruction and relaxation, by the appearance of surface electron states and resonances, the surface properties and related temperature scales of strongly correlated f-materials may differ dramatically from those in the bulk. Applying low energy electron and photoelectron diffraction techniques, momentum-resolved photoelectron spectroscopy and ab initio calculations, we demonstrate that the In-terminated surface of the heavyfermion superconductor CeIrIn5 experiences a reconstruction with a (root 2v x root 2)R45 degrees ordered structure. The latter appears due to the displacement of In atoms with respect to the Ir sublattice. We show that the electronic structure and related properties of the reconstructed In surface differ remarkably from the unreconstructed case. Namely, the predicted surface states with Rashba-type spin splitting do not appear. Our results suggest surface instabilities in similar quasi-two-dimensional strongly correlated f-materials, for which surface reconstructions can be unveiled by means of diffraction techniques.

Electronic structure

Ab initio calculations

Photoelectron diffraction

Atomic structure

Heavy fermion

Surface state

Author

Artem V. Tarasov

Saint Petersburg State University - Spsu

Max Mende

Technische Universität Dresden

Khadiza Ali

Chalmers, Microtechnology and Nanoscience (MC2), Quantum Device Physics

Georg Poelchen

Technische Universität Dresden

European Synchrotron Radiation Facility (ESRF)

Susanne Schulz

Technische Universität Dresden

oleg Yu. Vilkov

Saint Petersburg State University - Spsu

Kirill A. Bokai

Saint Petersburg State University - Spsu

Matthias Muntwiler

Paul Scherrer Institut

Vladislav Mandic

Goethe University Frankfurt

Clemens Laubschat

Technische Universität Dresden

Kristin Kliemt

Goethe University Frankfurt

Cornelius Krellner

Goethe University Frankfurt

Denis V. Vyalikh

Donostia International Physics Center

Basque Foundation for Science (Ikerbasque)

Dmitry Yu. Usachov

Saint Petersburg State University - Spsu

Surfaces and Interfaces

2468-0230 (ISSN)

Vol. 32 102126

Subject Categories

Materials Chemistry

Other Physics Topics

Condensed Matter Physics

DOI

10.1016/j.surfin.2022.102126

More information

Latest update

8/25/2022