Elastic and inelastic diffraction of fast neon atoms on a LiF surface
Journal article, 2023

Grazing incidence fast atom diffraction has mainly been investigated with helium atoms, considered as the best possible choice for surface analysis. This article presents experimental diffraction profiles recorded with neon projectile, between 300 eV and 4 keV kinetic energy with incidence angles theta i between 0.3 and 1.5 degrees along three different directions of a LiF(001) crystal surface. These correspond to perpendicular energy ranging from a few meV up to almost 1 eV. A careful analysis of the scattering profile allows us to extract the diffracted intensities even when inelastic effects become so large that most quantum signatures have disappeared. The relevance of this approach is discussed in terms of surface topology. We used the scattering profiles recorded along a random direction to deconvolute the diffraction profiles recorded along the [100] direction. The procedure was extended beyond the vertical dotted line corresponding to deeply inelastic conditions.

Author

Maxime Debiossac

University Paris-Saclay

Inst Quantum Technol

Peng Pan

Chalmers, Chemistry and Chemical Engineering, Energy and Material

Philippe Roncin

University Paris-Saclay

Physical Chemistry Chemical Physics

1463-9076 (ISSN) 1463-9084 (eISSN)

Vol. 45 25 30966-30974

Subject Categories

Atom and Molecular Physics and Optics

DOI

10.1039/d3cp04034h

PubMed

37937541

More information

Latest update

12/7/2023