Multifunctional thermoregulating and water repellent cellulosic textile
Journal article, 2025

Enhancing thermal comfort in textiles can contribute to improved user well-being, both in wearable technology and everyday clothing. This study introduces thermoregulation properties by embedding a phase change material (PCM) into regenerated man-made cellulose fibers via the Ioncell (R) technology. Calorimetric analysis revealed that the incorporation of myristic acid as PCM enables the fibers to absorb and release thermal energy, providing dynamic thermal regulation in response to temperature changes. Specifically, the PCM-fiber containing 50% (w/w) myristic acid demonstrated a phase change melting enthalpy of 73 J g-1, with a melting temperature of 54 degrees C. The melting enthalpy remained largely stable even after 100 thermal cycling tests, highlighting the excellent durability of the PCM-incorporated textiles. Furthermore, the resulting thermoregulating textile was treated with a hydrophobic coating composed of octadecenyl succinic anhydride, resulting in an average water contact angle of 75 degrees, after post-washing, demonstrating good water repellency. The developed fabric combines thermal regulation with water repellency through eco-friendly processes, offering a promising alternative to conventional functional textiles.

Shell

Phase-change materials

Starch

Myristic acid

Microencapsulation

Ioncell-F

Fibers

Thermal-energy storage

Author

Zahra Madani

Aalto University

Hossein Baniasadi

Aalto University

Pedro E. S. Silva

Aalto University

Maija Vaara

Aalto University

Marike Langhans

Aalto University

Inge Schlapp-Hackl

Aalto University

Lars Evenäs

Chalmers, Chemistry and Chemical Engineering, Applied Chemistry

Michael Hummel

Aalto University

Jaana Vapaavuori

Aalto University

Green Chemistry

1463-9262 (ISSN) 1463-9270 (eISSN)

Vol. In Press

Subject Categories (SSIF 2025)

Materials Chemistry

Textile, Rubber and Polymeric Materials

DOI

10.1039/d5gc00943j

PubMed

40386119

Related datasets

Multifunctional thermoregulating and water repellent cellulosic textile dataset [dataset]

URI: https://zenodo.org/records/15347991

More information

Latest update

5/28/2025