Flatband Resonance Enhanced Second-Harmonic Generation in Thin-Film Lithium Niobate Moire Microcavity
Other text in scientific journal, 2026

Optical nonlinear processes are fundamental to numerous applications, from frequency conversion to quantum technologies. Although subwavelength integrated photonic structures can enhance nonlinear interactions, they rarely exploit the broad oblique wavevector components of tightly focused pump beams, restricting the nonlinear conversion efficiency. Here, we demonstrate efficient second-harmonic generation (SHG) pumped by tightly focused beams containing broad oblique wavevector components in thin-film lithium niobate (TFLN) moire superlattice microcavity. Specifically, we experimentally achieve flatband enhanced SHG in a 4.41 degrees-twisted moire cavity with a high quality (Q) factor of similar to 1100 and a normalized SHG conversion efficiency of (2.1 +/- 0.4) & times; 10-4 cm2/GW at an extremely low pump power density of 1.1 +/- 0.2 MW/cm2. The synergy of high Q, flatband dispersion, and broad angular acceptance maximizes pump utilization, enabling high-efficiency nonlinear conversion. This breakthrough establishes TFLN moire superlattices as a versatile platform for compact, integrated nonlinear photonics and next-generation quantum light sources.

lithium niobate fabrication

moire flatband

second-harmonic generation

microcavity

Author

Zhuoran Hu

Shanghai Jiao Tong University

Zengya Li

Nano and Biophysics 1

Xingyao Huang

Shanghai Jiao Tong University

Hao Li

Shanghai Jiao Tong University

Bo Wang

Shanghai Jiao Tong University

Haigang Liu

Shanghai Jiao Tong University

Yuanlin Zheng

Shanghai Jiao Tong University

Xianfeng Chen

Shanghai Jiao Tong University

Shandong Normal University

Nano Letters

1530-6984 (ISSN) 1530-6992 (eISSN)

Vol. 26 22 7356-7363

Subject Categories (SSIF 2025)

Atom and Molecular Physics and Optics

Other Physics Topics

DOI

10.1021/acs.nanolett.6c01183

PubMed

42220042

More information

Latest update

6/25/2026