Solar hydrogen production with semiconductor metal oxides: new directions in experiment and theory
Reviewartikel, 2012
An overview of a collaborative experimental and theoretical effort toward efficient hydrogen production via photoelectrochemical splitting of water into di-hydrogen and di-oxygen is presented here. We present state-of-the-art experimental studies using hematite and TiO(2) functionalized with gold nanoparticles as photoanode materials, and theoretical studies on electro and photo-catalysis of water on a range of metal oxide semiconductor materials, including recently developed implementation of self-interaction corrected energy functionals.
rutile tio2(110) surface
reaction
electronic-structure
self-interaction correction
density-functional approximations
water oxidation
initio molecular-dynamics
oxygen evolution
total-energy calculations
effective core potentials
basis-set
wave
Författare
A. Valdes
CSIC - Instituto de Fisica Fundamental (IFF)
Gorlaeus Laboratories
J. Brillet
Ecole Polytechnique Federale de Lausanne (EPFL)
Michael Graetzel
Ecole Polytechnique Federale de Lausanne (EPFL)
H. Gudmundsdottir
Háskóli Íslands
H. A. Hansen
Danmarks Tekniske Universitet (DTU)
H. Jonsson
Stanford University
Háskóli Íslands
P. Klupfel
Háskóli Íslands
G. J. Kroes
Gorlaeus Laboratories
F. Le Formal
Ecole Polytechnique Federale de Lausanne (EPFL)
I. C. Man
Danmarks Tekniske Universitet (DTU)
Rafael Da Silva Martins
Chalmers, Teknisk fysik, Kemisk fysik
J. K. Norskov
Stanford University
J. Rossmeisl
Danmarks Tekniske Universitet (DTU)
K. Sivula
Ecole Polytechnique Federale de Lausanne (EPFL)
Aleksandra Vojvodic
Stanford University
Michael Zäch
Chalmers, Teknisk fysik, Kemisk fysik
Physical Chemistry Chemical Physics
1463-9076 (ISSN) 1463-9084 (eISSN)
Vol. 14 1 49-70Ämneskategorier
Fysikalisk kemi
DOI
10.1039/c1cp23212f