A Large Scale Multi-Modal Workflow for Battery Characterization: From Concept to Implementation
Artikel i vetenskaplig tidskrift, 2026
The development of material acceleration platforms in battery research requires integrating complementary techniques and correlating heterogeneous experimental datasets. Here, this challenge is addressed through a large-scale multimodal program involving fifteen European laboratories and facilities. Coordinated experiments on graphite/ (Formula presented.) Li-ion full cells address two scientific questions: is the electrolyte composition impacting electrode properties, and how do electrode materials evolve when cells are cycled to their end-of-life? A fully standardized workflow is demonstrated, from sample production and delivery, to metadata and data handling, generating seventy-five concatenated datasets shared among partners. Their integrated analysis reveals that scientific conclusions strongly depend on both the observable chosen to describe electrode properties, and the characterization technique employed. Beyond providing detailed insights into specific aspects as crystal structures, redox activity, surface processes or morphology, individual experiments can also act as binary diagnostic tool. Two-dimensional observable-technique patterns are introduced, where each pixel encodes a yes, no or uncertain answer to a scientific question. These multi-property metaviews enable the classification of material behavior and technique suitability according to user demand and criteria, highlighting the interdependence between measurement, extracted parameters, and scientific interpretation. This work establishes a proof-of-concept toward integrated and holistic battery research workflows.
aging
correlation
battery
experimental characterization
multi-modal
workflow
large scale
Författare
François Cadiou
European Synchrotron Radiation Facility (ESRF)
Université Grenoble Alpes
C. N. Herrera
Université Grenoble Alpes
Institut Laue-Langevin
Duncan Atkins
Institut Laue-Langevin
Elixabete Ayerbe
Centro de Investigacion Tecnológica En Electroquimica
Giorgio Baraldi
Centro de Investigacion Tecnológica En Electroquimica
Basquevolt
Stephanie Belin
SOLEIL Synchrotron
Anass Benayad
Université Grenoble Alpes
Didier Blanchard
European Synchrotron Radiation Facility (ESRF)
Federico G. Capone
RS2E
Sorbonne Université
Ennio Capria
European Synchrotron Radiation Facility (ESRF)
Isidora Cekic-Laskovic
Forschungszentrum Jülich
R. Dominko
Kemijski Inštitut
K. Edstrom
Uppsala universitet
Ajay Gautam
TU Delft
Lukas Helfen
Institut Laue-Langevin
A. Iadecola
RS2E
Sorbonne Université
Quentin Jacquet
Université Grenoble Alpes
Gregor Kapun
Kemijski Inštitut
Xinyu Li
Danmarks Tekniske Universitet (DTU)
Aleksandar Matic
Chalmers, Fysik, Materialfysik
Nataliia Mozhzhukhina
Chalmers, Fysik, Materialfysik
Andrew Naylor
Uppsala universitet
P. Norby
Danmarks Tekniske Universitet (DTU)
Chris O'Keefe
University of Cambridge
A. Ponrouch
Consejo Superior de Investigaciones Científicas (CSIC)
Jean Pascal Rueff
SOLEIL Synchrotron
Elena Tchernykova
Kemijski Inštitut
D. S. Tchitchekova
Consejo Superior de Investigaciones Científicas (CSIC)
Israel Temprano
University of Cambridge
Nikita Vostrov
European Synchrotron Radiation Facility (ESRF)
Marnix Wagemaker
TU Delft
Martin Winter
Forschungszentrum Jülich
Christian Wölke
Forschungszentrum Jülich
T. Vegge
Danmarks Tekniske Universitet (DTU)
Sandrine Lyonnard
Université Grenoble Alpes
Advanced Energy Materials
1614-6832 (ISSN) 1614-6840 (eISSN)
Vol. In PressBattery Interface Genome - Materials Acceleration Platform - BIG-MAP
Europeiska kommissionen (EU) (EC/H2020/957189), 2020-09-01 -- 2023-08-31.
Ämneskategorier (SSIF 2025)
Atom- och molekylfysik och optik
Energiteknik
Teknisk mekanik
Drivkrafter
Hållbar utveckling
Styrkeområden
Energi
DOI
10.1002/aenm.71288