Accelerating Plasmonic Hydrogen Sensors for Inert Gas Environments by Transformer-Based Deep Learning
Journal article, 2025

Rapidly detecting hydrogen leaks is critical for the safe large-scale implementation of hydrogen technologies. However, to date, no technically viable sensor solution exists that meets the corresponding response time targets under technically relevant conditions. Here, we demonstrate how a tailored long short-term transformer ensemble model for accelerated sensing (LEMAS) speeds up the response of an optical plasmonic hydrogen sensor by up to a factor of 40 and eliminates its intrinsic pressure dependence in an environment emulating the inert gas encapsulation of large-scale hydrogen installations by accurately predicting its response value to a hydrogen concentration change before it is physically reached by the sensor hardware. Moreover, LEMAS provides a measure for the uncertainty of the predictions that are pivotal for safety-critical sensor applications. Our results advertise the use of deep learning for the acceleration of sensor response, also beyond the realm of plasmonic hydrogen detection.

nanoparticles

deep learning

hydrogen sensing

neural networks

plasmonic sensing

Author

Viktor Martvall

Chalmers, Physics, Condensed Matter and Materials Theory

Henrik Klein Moberg

Chalmers, Physics, Chemical Physics

Athanasios Theodoridis

Chalmers, Physics, Chemical Physics

David Tomecek

Chalmers, Physics, Chemical Physics

Pernilla Ekborg-Tanner

Chalmers, Physics, Condensed Matter and Materials Theory

Sara Nilsson

Chalmers, Physics, Chemical Physics

Giovanni Volpe

University of Gothenburg

Paul Erhart

Chalmers, Physics

Christoph Langhammer

Chalmers, Physics, Chemical Physics

ACS Sensors

23793694 (eISSN)

Vol. In Press

Analysis and Modelling Service for Engineering Materials Studied with Neutrons

Swedish Research Council (VR) (2018-06482), 2018-11-01 -- 2020-12-31.

hAIdrogen safety sensors

VINNOVA (2021-02760), 2021-10-25 -- 2024-10-24.

Phase behavior and electronic properties of mixed halide perovskites from atomic scale simulations

Swedish Research Council (VR) (2020-04935), 2020-12-01 -- 2024-11-30.

Subject Categories (SSIF 2025)

Atom and Molecular Physics and Optics

Condensed Matter Physics

Areas of Advance

Nanoscience and Nanotechnology

Infrastructure

Chalmers Materials Analysis Laboratory

Nanofabrication Laboratory

Chalmers e-Commons

DOI

10.1021/acssensors.4c02616

More information

Latest update

1/16/2025